I'm not really into movie soundtracks because they usually suck but I would have to say that the Garden State Soundtrack is the best. I listen to it allot & I love every song, Its almost perfect.
"Don't Panic" - Coldplay
"Caring Is Creepy" - The Shins
"In the Waiting Line" - Zero 7
"New Slang" - The Shins
"I Just Don't Think I'll Ever Get Over You" - Colin Hay
"Blue Eyes" - Cary Brothers
"Fair" - Remy Zero
"One of These Things First" - Nick Drake
"Lebanese Blonde" - Thievery Corporation
"The Only Living Boy in New York" - Simon & Garfunkel
"Such Great Heights" - Iron & Wine
"Let Go" - Frou Frou
"Winding Road" - Bonnie Somerville
